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1 Such pulses lead to a new regime of laser matter interaction, the nonlinear, nonperturbative regime. 5 At the very high intensities now available, I t 1014 W/cm2, one now must consider dissociative ionization so that one must deal with boundcontinuum transitions both in the electronic and nuclear Hilbert space. 4 Inclusion of ionization involves treating numerically the complete field-electron-nuclear non-Born-Oppenheimer problem. 10,11 Electronic interaction with radiation in molecules differs from that of atoms because of the large delocalization of electrons in the former.

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